Welcome to TFP!!!
What is your CH? That is likely scale...if it is rough. If it is smooth, likely a bleached liner...who knows why? Really weird...as calcium scale like this is RARE in a vinyl pool. If it is calcium scale, your level of calcium scale is impressive. My guess is previous owner used Cal-Hypo to chlorinate and your CH is
VERY high.
How are you testing? Looks like pool store test results. I would get a good test kit POST HASTE...to get a good bead on your CH levels. Link-->
Test Kits Compared
By lowering PH and maintaining a lower pH, you may be able to eventually get the scale off, but it can take a
very long time. Plus if the CH level gets too high, which it may already be, and which it will eventually be high again (as you are removing the calcium scale), it will stop working until you replace water to get CH back down. Also it is important to not lower PH below 6.8 as that will damage the liner. Will require a dance between keeping pH low and regular replacement of lower CH water.
If the scaling is especially bad, like yours, most people end up replacing the liner...and may be the easiest route to a Trouble Free Pool. How big is the pool?
In some cases it is possible to physically remove the scale and dispose of it. The challenge is to do this without damaging the liner. Likely difficult in your situation with the embossing on the liner.
You might try this....
with diluted acid to dissolve the calcium. The risk is in the dilution to remove the scale without bleaching the liner. The struggle will be that amount of calcium that you have (assuming it is calcium scale), as it will take a lot of work.
You are in a pickle. I love a good pickle...just not this kind. I'm sorry for your situation.