Pool School here has a lot more about it, but essentially, the more CYA you have, the higher your FC level must be to remain effective. Since tablets add CYA, it increases over time, and if you up the output of the chlorinator it just adds more, faster. To the point where it is unsustainable.
So at 100 - you need lots of FC in your water.
Below is the chart as to what levels to be at, based on CYA amounts, in ppm terms.
The Minimum is just that, and at that level, you are in danger of dipping too low between tests and allowing algae to grow.
Note that, unfortunately, above levels of 9-10ppm FC, the pH test becomes unreliable. So also a problem measuring that.
The SLAM section is what you have to bring your FC level to, for a sustained period (days, many days) to kill off existing algae.
In simplistic terms, the CYA absorbs a lot of the FC (that still shows up in your tests, but is not active). As you loose FC, some of that absorbed FC is released back and becomes active again. Hence why some CYA is good - it acts as a buffer from going too low. But there are limits as to what it will give back.
Salt water generators are much more consistent in replenishing CL, so one can run at lower levels, with less risk of going too low. But they aren't good at rapidly increasing levels, hence why the recommendation to run with a higher CYA level than a pool without one.
The only way to reduce CYA is to replace the water with fresh.
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