No wrong per se...just making it all a little more complicated than needed...those instructions are for temporary seasonal pools (you know, like intex), which are usually much smaller, so the benefit of the dichlor bags for them would be they'd be more cost effective than buying that big 4lb container of stabilizer and then using using a teensy fraction of the bottle. Nonetheless, you *can* add your CYA that way...but it seems much more protracted at 27,000 gallons -- and your chlorine will be "unbuffered" all that time. And it could be as much as a week after your LAST DOSE to have a TRUE CYA reading! Which would make that 3 weeks out...
If you already have the dichlor, carry on, as there's no point spending more money than you need to. But if you haven't bought the dichlor yet, why not just use the CYA granules you need, use pool calc to determine exact dose, then forget-about-it for a week or so...longer in cold water...to even get a read (it will take longer to dissolve).
When you say you could not get it below 100, do you mean when you drained it earlier? Or are you just saying that you don't yet know if your reading is accurate -- eg. could be considerably higher right now?
What is your water level right now, and your CYA level right now? What I meant was why buy more CYA and try to dose it when you could just approximate how much MORE water you need to drain/change to get the right amount of CYA that's in your water already!
Eg. if you're at 100 ppm cya right now and the pool is 3/4 full...drain 2 more quarters, fill er up, and read your CYA -- should come in around 33! At 27,000 gallons, I'm thinking that should save you about $45 -- or if you were using the liquid, more like $100+.
And if the readings wrong, well, just drain more
Just trying to help you simplify it. The fact that your CYA got to well over 100 means you've developed a reliance on those stabilized products and you now need to kind of train yourself to think a little differently -- eg "I need just this, so I'll add just this..." "I need to always measure my FC, not just assume adding one pack of blabity blah"..."I will avoid adding hybrid products so that I can get comfortable with controlling specific variables..." etc. You know, BBB pool-owner affirmations